Dose-dependent effects of MIL-88A(Fe) and MIL-101(Fe) on arsenic immobilization and phytoremediation using ramie (Boehmeria nivea L.)
文献类型： 外文期刊
作者： Ye, Jian 1 ; Yin, Xingyan 1 ; Yang, Chunping 1 ; Tan, Xiaofei 1 ; Li, Chuang 1 ; Chen, Gaobin 1 ; Chen, Ping 6 ; Chen, Qiang 1 ; Dai, Mingyang 1 ;
作者机构： 1.Hunan Univ, Coll Environm Sci & Engn, Changsha 410082, Peoples R China
2.Hunan Univ, Key Lab Environm Biol & Pollut Control, Minist Educ, Changsha 410082, Peoples R China
3.Hunan Univ, Shenzhen Res Inst, Shenzhen 518055, Peoples R China
4.Hainan Univ, Sch Environm Sci & Engn, Key Lab Agroforestry Environm Proc & Ecol Regulat, Haikou 570228, Hainan, Peoples R China
5.Guangdong Univ Petrochem Technol, Acad Environm & Resource Sci, Sch Environm Sci & Engn, Maoming 525000, Guangdong, Peoples R China
6.Chinese Acad Agr Sci, Inst Bast Fiber Crops, Changsha 410205, Hunan, Peoples R China
关键词： Metal-organic framework (MOF); Ramie phytoremediation; Soil remediation; As bioavailability; Microbial community
期刊名称：CHEMICAL ENGINEERING JOURNAL （ 影响因子：13.2； 五年影响因子：13.5 ）
ISSN： 1385-8947
年卷期： 2025 年 517 卷
页码：
收录情况： SCI
摘要： The efficacy and environmental effects of using metal-organic frameworks (MOFs) for the remediation of arsenic (As)-contaminated soil, a significant global problem, remain unclear. This study evaluated MIL-88A(Fe) and MIL101(Fe) coupled with ramie (Boehmeria nivea L.) for As-contaminated soil remediation. A soil incubation experiment revealed that 10,000 mg kg-1 MIL-88A(Fe) and MIL-101(Fe) reduced As bioavailability by 77.1 % and 65.0 %, respectively, and increased residual As fractions by 8 % and 7 % through Fe-As co-precipitation and adsorption. Divergent environmental effects emerged, which were probably due to differences in the framework structures and organic ligands: MIL-88A(Fe) improved soil urease activity and bacterial diversity, whereas MIL101(Fe) induced acidification (decreasing soil pH by 25 %) and salinity stress (elevating soil electrical conductivity (EC) by 946 %). A pot experiment showed that 1000 mg kg-1 MOFs enhanced ramie biomass via As immobilization, whereas 5000 mg kg-1 MIL-101(Fe) suppressed growth because exposure to the MOF caused root damage. The MOFs enriched Pseudomonas (As-oxidizing) and suppressed Dokdonella (pathogenic), enhancing plant resilience. Notably, 100 mg kg-1 MIL-101(Fe) increased As translocation to stems (14.8 %) and leaves (27.6 %). Hydroponic analyses showed that 50-200 mg L-1 MIL-101(Fe) mitigated As-induced chlorophyll degradation (elevating Soil and plant analyzer development (SPAD) by 12.8 %-28.3 %), whereas 500 and 1000 mg L-1 induced oxidative stress (reducing SPAD by 4.2 %-10.7 %). This study provides valuable insights into using Fe-based MOFs in soil remediation and highlights their beneficial and harmful effects.
- 相关文献
作者其他论文 更多>>
-
Chitooligosaccharide application enhanced the growth and phytoremediation efficiency of industrial hemp in Cd-contaminated soils
作者：Guo, Yuan;Zhao, Xinlin;Wang, Yuanchang;Wang, Chenyuan;Zhou, Wei;Huang, Rong;Guo, Yuan;Zhao, Xinlin;Wang, Yuanchang;Wang, Chenyuan;Zhou, Wei;Huang, Rong;Guo, Yuan;Zhao, Xinlin;Ouyang, Da;Gao, Shuaishuai;Tan, Xiaofei;Tan, Xiaofei;Tan, Xiaofei
关键词：Antioxidant; Bioconcentration; Biomass; Cannabis sativa; Heavy metal; Phytomanagement
-
Soybean-maize intercropping combined with water management enhances leaf traits to obtain yield benefits in semi-arid regions
作者：Chen, Ping;Xian, Gaojie;Pu, Tian;Yang, Feng;Wang, Xiaochun;Yong, Taiwen;Li, Yuze;Yang, Wenyu;Wu, Yushan;Chen, Ping;Xian, Gaojie;Pu, Tian;Yang, Feng;Wang, Xiaochun;Yong, Taiwen;Li, Yuze;Yan, Yanhong;Liu, Jiang;Yang, Wenyu;Wu, Yushan;Chen, Ping;Gong, Wanzhuo;Li, Jianzheng;Yan, Yanhong;Liu, Jiang
关键词：Cropping system; Photosynthetic plasticity; Productivity; Competition; Economic benefits
-
The CsphyB-CsPIF4-CsBRC1 module regulates ABA biosynthesis and axillary bud outgrowth in cucumber
作者：Liu, Ye;Liu, Zhihan;Li, Chuang;Li, Min;She, Daixi;Zhang, Jiahao;Ren, Huiqi;Zhong, Xitong;Huang, Yafei;Huang, Yuxiang;He, Yuting;Liu, Yuan;Chen, Jiacai;Geng, Yan;Zhang, Xiaolan;Zhao, Jianyu;Li, Xiaoli;Bo, Kailiang;Weng, Yiqun;Weng, Yiqun
关键词：ABA; axillary bud outgrowth; CsBRC1; CsphyB; CsPIF4; cucumber
-
Substrate-based discovery of α-hydroxycarboxylic acid derivatives as potential herbicides targeting dihydroxyacid dehydratase
作者：He, Bo;Hu, Yanhao;He, Xu;Chen, Wang;Feng, Mingfeng;Chen, Ping;Wei, Lirong;Li, Yu;Yan, Wei;Li, Jun;Feng, Zhike;Ye, Yonghao;Liu, Dongshan;Zang, Xin;Zhou, Jiahai;Yang, Jingfang;Zhou, Jiahai
关键词：
-
Advances in Starch-Based Nanocomposites for Functional Food Systems: Harnessing AI and Nuclear Magnetic Resonance Technologies for Tailored Stability and Bioactivity
作者：Sun, Yue;Wang, Ziyu;Ye, Jian;Cao, Ruge;Li, Yinta;Wang, Lili
关键词：starch-based nanocomposites (SNCs); artificial intelligence (AI); nuclear magnetic resonance (NMR); predictive modeling; food matrix
-
Nanoparticles for improving biogas production and effluent biofertilizer
作者：Abdelwahab, Taha Abdelfattah Mohammed;Darwish, Elwan Ali;Desoky, Samir Hafez Mohamed;Fodah, Ahmed Elsayed Mahmoud;Pan, Junting;Ni, Ji-Qin;Yang, Chunping;Yang, Chunping;Yang, Chunping;Mohanty, Mahendra Kumar;Yang, Haiping;Fodah, Ahmed Elsayed Mahmoud
关键词：Anaerobic digestion; Digestate; Kinetic model; Fertilizer; Nanoparticle mixture
-
International research initiative on genomics-guided sugarcane breeding
作者：Zhang, Xingtan;Wang, Jungang;Que, Youxiong;Lin, Jishan;Zhang, Xingtan;Noor-ul-Ain;Abid, Javeria;Wang, Ren;Zhang, Jisen;Bao, Yixue;Zhang, Muqing;Zhang, Jisen;Bao, Yixue;Zhang, Muqing;Zhao, Peifang;Zhang, Yuebin;Chen, Li-yu;Ming, Ray;Herry, Robert;Tangphatsornruang, Sithichoke;Wang, Qinnan;Wang, Qinnan;Huang, Dongliang;Ye, Jian;Luo, Ming;Butterfield, Mike
关键词：
