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The spatio-temporal variability of soil microplastic distribution and erosion-induced microplastic export under extreme rainfall event using sediment fingerprinting and 7Be in intensive agricultural catchment

文献类型： 外文期刊

作者： Chen, Xiaoyan 1 ; Lu, Zhaoyang 1 ; Heng, Lee 2 ; Chappell, Adrian 3 ; Oshunsanya, Suarau Odutola 1 ; Adu-Gyamfi, Joseph 2 ; Liu, Wenxiang 1 ; Yu, Hanqing 1 ;

作者机构： 1.Chinese Acad Agr Sci CAAS, Inst Environm & Sustainable Dev Agr, Beijing 100081, Peoples R China

2.IAEA, Vienna, Austria

3.Cardiff Univ, Sch Earth & Environm Sci, Cardiff, Wales

4.Univ Ibadan, Dept Soil Resources Management, Ibadan, Nigeria

5.Changjiang River Sci Res Inst, Chongqing Branch Inst, Chongqing 400026, Peoples R China

关键词： Microplastic; Spatio-temporal variability; Compound specific stable isotope (CSSI); Berillium-7; Export loads

期刊名称：JOURNAL OF HAZARDOUS MATERIALS （ 影响因子：11.3； 五年影响因子：12.4 ）

ISSN： 0304-3894

年卷期： 2025 年 488 卷

页码：

收录情况： SCI

摘要： Intensive agricultural production and land management often lead to soil microplastics (MPs) accumulation and aggravated erosion consequently polluting water bodies. However, little is known about the occurrence and migration of soil MPs induced by soil erosion at the catchment scale. This study firstly reported the spatio-temporal variability in soil MPs distribution, and erosion-induced microplastic export loads under extreme rainfall events in an intensive agricultural catchment. The results indicated that microplastic abundance peaked in November 2022 and varied by land use types, among which cropland converted from forest (C(F)) and crop farmland (C) had the highest abundance, vegetable farmland (V) had the lowest abundance on average. Most MPs were < 500 mu m and the primary polymers were polyamide (PA), polypropylene (PP) and polyethylene (PE). Sediment contribution and microplastic export loads were identified using compound specific stable isotope and Berillium-7 under an extreme rainfall event. F and C(F) were merged because their delta C-13 values were non-distinguishable and were identified as the primary sediment source (50.14 +/- 0.27 %), contributing most to microplastic export loads due to land management policy shifting. Changed land uses should be the main focus for catchment erosion control and microplastic pollution prevention in intensive agriculture in China and elsewhere.

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