Effect of straw decomposition on hexavalent chromium removal by straw: Significant roles of surface potential and dissolved organic matter
文献类型： 外文期刊
作者： Xia, Xing 1 ; Zhang, Xingbin 1 ; Liu, Peng 1 ; Zhang, Yongyi 1 ; Hou, Tingting 1 ; Zhang, Ranran 1 ; He, Jiehong 1 ; Fang, Guodong 3 ; Yang, Jianjun 4 ; Wu, Xiangwei 1 ;
作者机构： 1.Anhui Agr Univ, Coll Resources & Environm, Anhui Prov Key Lab Hazardous Factors & Risk Contro, Hefei 230036, Peoples R China
2.Anhui Agr Univ, Coll Resources & Environm, Anhui Prov Key Lab Farmland Ecol Conservat & Pollu, Hefei 230036, Peoples R China
3.Chinese Acad Sci, Inst Soil Sci, Key Lab Soil Environm & Pollut Remediat, Nanjing 210008, Peoples R China
4.Chinese Acad Agr Sci, Inst Agr Resources & Reg Planning, State Key Lab Efficient Utilizat Arid & Semiarid A, Beijing 100081, Peoples R China
关键词： Heavy metal; Straw return; Straw decomposition; Adsorption; XAS
期刊名称：JOURNAL OF COLLOID AND INTERFACE SCIENCE （ 影响因子：9.7； 五年影响因子：8.9 ）
ISSN： 0021-9797
年卷期： 2025 年 678 卷
页码：
收录情况： SCI
摘要： Mobility and bioavailability of hexavalent chromium (Cr(VI)) in agricultural soils are affected by interactions between Cr(VI) and returned crop straws. However, the effect of straw decomposition on Cr(VI) removal and underlying mechanisms remain unclear. In this study, Cr(VI) removal by pristine and decomposed rice/rape straws was investigated by batch experiments and a series of spectroscopies. The results showed that straw decomposition inhibited Cr(VI) removal, regardless of straw types. However, the potential mechanisms of the inhibition were distinct for the two straws. For the rice straw, a lower zeta potential after decomposition suppressed Cr(VI) sorption and subsequent reduction. In addition, less Cr(VI) was reduced by the decomposed rice straw-derived dissolved organic matter (DOM) than the pristine one. In contrast, for the rape straw, due to the increased zeta potential after decomposition, the decreased Cr(VI) removal was mainly ascribed to less Cr(VI) reduction by the rape straw-derived DOM. These results emphasized the significant roles of straw surface potential and DOM in Cr(VI) removal, depending on straw types and decomposition, which facilitate the fundamental understanding of Cr(VI) removal by straws and are helpful for predicting the environmental risk of Cr and rational straw return in Cr(VI)-contaminated fields.
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