Room temperature agricultural ethylene detection by freestanding three-dimensional porous-ZnO/carbon nanofibers
文献类型： 外文期刊
作者： Li, Xian 1 ; Xu, Chengcheng 2 ; Sun, Jie 2 ; Long, Yin 2 ; Wang, Yang 2 ; Li, Zhemin 1 ; Bai, Chunjiang 4 ; Du, Xiaosong 2 ;
作者机构： 1.Chinese Acad Agr Sci, Agr Informat Inst, Beijing 100081, Peoples R China
2.Univ Elect Sci & Technol China, Sch Optoelect Sci & Engn, State Key Lab Elect Thin Films & Integrated Device, Chengdu 610054, Peoples R China
3.Chinese Acad Agr Sci, Grad Sch, Beijing 100081, Peoples R China
4.China Acad Space Technol Xian, Natl Key Lab Sci & Technol Space Microwave, Xian 710100, Peoples R China
关键词： Ethylene sensor; Porous nanofibers network; Electrospinning; Synergistic effect
期刊名称：SENSORS AND ACTUATORS B-CHEMICAL （ 影响因子：8.4； 五年影响因子：7.2 ）
ISSN：
年卷期： 2024 年 398 卷
页码：
收录情况： SCI
摘要： Ethylene is one of the important indicators to reflect the ripeness and senescence of the fruit. Ethylene sensor can be applied for fast ethylene detection nondestructively, yet high temperature condition of the common metal oxide semiconductors restrains its agricultural applications. Herein, porous-ZnO/carbon nanofibers (CNFs) three-dimensional structure, derived from Zeolite imidazole framework-8 (ZIF-8) /polyacrylonitrile (PAN) electrospun nanofibers, was proposed and further optimized. The results showed that porous-ZnO/CNFs exhibited increasing resistance to reducing ethylene at room temperature, well explained by the Fermi levels' relative position of the sensing system. Repeatability, selectivity and stability were demonstrated. The addition of porous-ZnO (10 % composting mass ratio) resulted in a 428 % increase in the ethylene-sensing response compared with CNFs, and a 64.2 % improvement compared with ZnO/CNFs. The outstanding sensing performance can be attributed to the synergistic effect of porous and interconnected morphology, the formed p-n heterojunction, as well as oxygen-vacancy effect. This strategy is beneficial for designing efficient gas sensors at room temperature, and exploring the application of the advanced gas sensors in intelligent agriculture field.
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