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Emerging applications of deep eutectic solvents in the preparation and functionalization of biomass-derived carbonaceous materials: challenges and prospects

文献类型： 外文期刊

作者： Shen, Yiyi 1 ; Zhou, Haiqin 1 ; He, Xiaotong 1 ; Shen, Feng 3 ; Xu, Zhixiang 4 ; Yang, Bo 5 ; Kong, Lingzhao 6 ; Dai, Lichun 1 ;

作者机构： 1.Minist Agr & Rural Affairs, Biogas Inst, Key Lab Dev & Applicat Rural Renewable Energy, Chengdu 610041, Sichuan, Peoples R China

2.Chinese Acad Agr Sci, Res Ctr Rural Energy & Ecol, Chengdu 610041, Sichuan, Peoples R China

3.Chinese Acad Agr Sci, Agroenvironm Protect Inst, 31 Fukang Rd, Tianjin 300191, Peoples R China

4.Jiangsu Univ, Sch Energy & Power Engn, Zhenjiang 212013, Peoples R China

5.Sanya Univ, Zhai Mingguo Academician Work Stn, Sanya 572022, Peoples R China

6.Suzhou Univ Sci & Technol, Sch Environm Sci & Engn, Suzhou 215009, Peoples R China

期刊名称：GREEN CHEMISTRY （ 影响因子：9.3； 五年影响因子：9.3 ）

ISSN： 1463-9262

年卷期： 2024 年 26 卷 14 期

页码：

收录情况： SCI

摘要： Biomass-derived carbonaceous materials (BCMs) have been extensively applied in diverse areas, attributed to their recognized sustainability, low cost, diverse and scalable synthesis routes, and tunable structure and function. Recently, deep eutectic solvents (DESs), a class of novel and green solvents, have emerged as a promising alternative to traditional solvents and processing techniques for the preparation and functionalization of BCMs for various applications. However, there is still a knowledge gap regarding the applications of DESs in the preparation and functionalization of BCMs. Considering these, this review summarizes the emerging applications of DESs in the preparation and functionalization of BCMs, including their use as biomass pretreatment solvents, carbon precursors, soft templates, solvothermal carbonization (STC) media, and post-modification agents. This review also discusses the applications of the resultant BCMs in various fields, such as pollution control, energy storage, and biocatalysis, and highlights the challenges and prospects for using DESs in the preparation and functionalization of BCMs. Overall, the use of designer DESs in the preparation and functionalization of BCMs has the potential to contribute to the development of sustainable and cost-effective technologies for a wide range of applications. Deep eutectic solvents can be used as the pretreatment solvents, carbon precursors, soft templates, carbonization media, and post-modification agents for the preparation and functionalization of biomass-derived carbonaceous materials.

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