"Memory catalysis": Extending the photocatalytic antibacterial performance of a palladium-modified ZnO nanocomposite
文献类型: 外文期刊
作者: Zhang, Jingtao 1 ; Zhu, Mengzhen 1 ; Liu, Shurui 1 ; Zhai, Mengwan 1 ; Yao, Jing 1 ; Wang, Guanghui 2 ; Li, Junyang 3 ; Perego, Patrizia 3 ; Sun, Xiaodong 4 ; Liu, Bingkun 2 ;
作者机构: 1.Zhengzhou Univ Light Ind, Sch Food & Bioengn, Zhengzhou 450002, Peoples R China
2.Zhengzhou Univ Light Ind, Sch Mat & Chem Engn, Zhengzhou 450002, Peoples R China
3.Univ Genoa, Dept Civil Chem & Environm Engn DICCA, Via Opera Pia 15, I-16145 Genoa, Italy
4.Hainan Acad Agr Sci, Inst Vegetables, Key Lab Vegetable Biol Hainan Prov, Haikou 571100, Hainan, Peoples R China
5.Luohe Weilong Biotechnol Co Ltd, Luohe 462000, Peoples R China
6.136 Kexue Rd, Zhengzhou, Henan, Peoples R China
关键词: PdO-ZnO nanocomposite; Photocatalysis; Antibacterial; Optical "memory"; Cytotoxicity test
期刊名称:JOURNAL OF WATER PROCESS ENGINEERING ( 影响因子:7.0; 五年影响因子:6.7 )
ISSN: 2214-7144
年卷期: 2023 年 54 卷
页码:
收录情况: SCI
摘要: In this study, Pd-ZnO nanocomposite was synthesized via the facile solvothermal method. Then, PdO-ZnO was obtained by continuing calcination of the synthesized Pd-ZnO. X-ray Diffraction (XRD), Transmission Electron Microscope (TEM), and X-ray Photoelectron Spectroscopy (XPS) tests showed that Pd was converted to PdO in the process of calcination. The photocatalytic sterilization experiment showed that in the 3 % Pd-ZnO system, 2 x 107 CFU/mL of E. coli was completely killed within 3 h, while 3 % PdO-ZnO took 1.5 h. In electron spin resonance (ESR) tests on PdO-ZnO, The & BULL;OH and & BULL;O2- signals can be detected under light and within 20 min after the end of light. 1 x 105 CFU/mL of E. coli were killed within 1 h by the optical "memory" effect of PdO-ZnO. PdO-ZnO inactivates E. coli by disrupting the membrane structure of bacteria as demonstrated by scanning electron microscopy (SEM) test. PdO-ZnO is non-toxic and can be demonstrated through cytotoxicity experiments on HTT2.
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